IPA: /ˌʌn.səkˈsɛf.əl.i/
KK: /ʌnˈsʌksɛsfəli/
In a way that does not achieve the desired result or goal.
She tried to fix the car, but she did it unsuccessfully.
Unsuccessfully → It is formed from "un-" (meaning not) and "success" (from Latin "successus", meaning to come close or to follow after) and the suffix "-fully" (meaning in a manner). The word "unsuccessfully" means in a manner that does not achieve success.
Think of 'not' ('un-') achieving 'success' — that's why 'unsuccessfully' means not achieving success.